Methane‑to‑methanol conversion and power co‑generation on palladium

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dc.contributor.authorCOELHO, JESSICA F.pt_BR
dc.contributor.authorFILHO, NIVALDO G.P.pt_BR
dc.contributor.authorGUTIERREZ, ISABELY M.pt_BR
dc.contributor.authorGODOI, CAMILA M.pt_BR
dc.contributor.authorGOMES, PAULO V.R.pt_BR
dc.contributor.authorZAMBIAZI, PRISCILLA J.pt_BR
dc.contributor.authorSOUZA, RODRIGO F.B. dept_BR
dc.contributor.authorNETO, ALMIR O.pt_BR
dc.coverageInternacionalpt_BR
dc.date.accessioned2022-12-16T18:55:06Z
dc.date.available2022-12-16T18:55:06Z
dc.date.issued2022pt_BR
dc.description.abstractThe use of palladium nickel catalysts with different compositions supported metal oxides, such as Sb2O5·SnO2 (ATO) catalyst combinations were employed to convert the methane-to-methanol in mild conditions using a fuel cell polymer electrolyte reactor. The catalysts used for the conversion of methane to methanol were characterized by XRD and observed the phases of ATO, the face-centered cubic structure of the Pd and Ni phases. All nanoparticles have a mean size between 9 and 12 nm as measured by TEM images. The products obtained from the methane oxidation, such as methanol and formate, were monitored using FT-IR spectroscopy to qualify the products formation, while High-Performance Liquid Chromatography was used to quantify them. In these studies, it was observed that as the electrical potential of the reactor increases, the generation of products decreases. The best results for the conversion of methane into methanol and energy co-generation were obtained from Pd50Ni50/ATO.pt_BR
dc.description.sponsorshipConselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq)pt_BR
dc.description.sponsorshipFundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)pt_BR
dc.description.sponsorshipIDCNPq: 302709/2020-7pt_BR
dc.description.sponsorshipIDFAPESP: 17/11937-4pt_BR
dc.format.extent5155-5168pt_BR
dc.identifier.citationCOELHO, JESSICA F.; FILHO, NIVALDO G.P.; GUTIERREZ, ISABELY M.; GODOI, CAMILA M.; GOMES, PAULO V.R.; ZAMBIAZI, PRISCILLA J.; SOUZA, RODRIGO F.B. de; NETO, ALMIR O. Methane‑to‑methanol conversion and power co‑generation on palladium: nickel supported on antimony tin oxide catalysts in a polymeric electrolyte reactor‑fuel cell (PER‑FC). <b>Research on Chemical Intermediates</b>, v. 48, n. 12, p. 5155-5168, 2022. DOI: <a href="https://dx.doi.org/10.1007/s11164-022-04857-9">10.1007/s11164-022-04857-9</a>. Disponível em: http://repositorio.ipen.br/handle/123456789/33470.
dc.identifier.doi10.1007/s11164-022-04857-9pt_BR
dc.identifier.fasciculo12pt_BR
dc.identifier.issn0922-6168pt_BR
dc.identifier.orcid0000-0001-8745-3421pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-9287-6071
dc.identifier.percentilfi52pt_BR
dc.identifier.percentilfiCiteScore69pt_BR
dc.identifier.urihttp://repositorio.ipen.br/handle/123456789/33470
dc.identifier.vol48pt_BR
dc.relation.ispartofResearch on Chemical Intermediatespt_BR
dc.rightsopenAccesspt_BR
dc.subjectmethane
dc.subjectconversion
dc.subjectenergy conversion
dc.subjecttransition elements
dc.subjectpalladium
dc.subjectnickel
dc.subjectfuel cells
dc.titleMethane‑to‑methanol conversion and power co‑generation on palladiumpt_BR
dc.typeArtigo de periódicopt_BR
dspace.entity.typePublication
ipen.autorNIVALDO GOMES PEREIRA FILHO
ipen.autorCAMILA MARINHO GODOI SANTOS
ipen.autorPRISCILLA JUSSIANE ZAMBIAZI
ipen.autorALMIR OLIVEIRA NETO
ipen.autorRODRIGO FERNANDO BRAMBILLA DE SOUZA
ipen.autorPAULOVICTORRODRIGUESGOMES
ipen.autorISABELY MAMMANA GUTIERREZ
ipen.autorJESSICA FERNANDA COELHO
ipen.codigoautor14974
ipen.codigoautor14128
ipen.codigoautor15708
ipen.codigoautor3541
ipen.codigoautor11260
ipen.codigoautor15526
ipen.codigoautor15839
ipen.codigoautor15191
ipen.contributor.ipenauthorNIVALDO GOMES PEREIRA FILHO
ipen.contributor.ipenauthorCAMILA MARINHO GODOI SANTOS
ipen.contributor.ipenauthorPRISCILLA JUSSIANE ZAMBIAZI
ipen.contributor.ipenauthorALMIR OLIVEIRA NETO
ipen.contributor.ipenauthorRODRIGO FERNANDO BRAMBILLA DE SOUZA
ipen.contributor.ipenauthorPAULOVICTORRODRIGUESGOMES
ipen.contributor.ipenauthorISABELY MAMMANA GUTIERREZ
ipen.contributor.ipenauthorJESSICA FERNANDA COELHO
ipen.date.recebimento22-12
ipen.identifier.fi3.3pt_BR
ipen.identifier.fiCiteScore5.5pt_BR
ipen.identifier.ipendoc29104pt_BR
ipen.identifier.iwosWoSpt_BR
ipen.identifier.ods7
ipen.range.fi3.000 - 4.499
ipen.range.percentilfi50.00 - 74.99
ipen.subtitulonickel supported on antimony tin oxide catalysts in a polymeric electrolyte reactor‑fuel cell (PER‑FC)pt_BR
ipen.type.genreArtigo
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sigepi.autor.atividadeNETO, ALMIR O.:3541:610:Npt_BR
sigepi.autor.atividadeSOUZA, RODRIGO F.B. de:11260:610:Npt_BR
sigepi.autor.atividadeZAMBIAZI, PRISCILLA J.:15708:610:Npt_BR
sigepi.autor.atividadeGOMES, PAULO V.R.:15526:720:Npt_BR
sigepi.autor.atividadeGODOI, CAMILA M.:14128:610:Npt_BR
sigepi.autor.atividadeFILHO, NIVALDO G.P.:14974:610:Npt_BR
sigepi.autor.atividadeCOELHO, JESSICA F.:15191:610:Spt_BR
sigepi.autor.atividadeGUTIERREZ, ISABELY M.:15839:610:N
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