Methane conversion to higher value‑added product and energy co‑generation using anodes OF PdCu/C in a solid electrolyte reactor

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dc.contributor.authorGODOI, C.M.pt_BR
dc.contributor.authorSANTOS, M.C.L.pt_BR
dc.contributor.authorSILVA, A.J.pt_BR
dc.contributor.authorTAGOMORI, T.L.pt_BR
dc.contributor.authorRAMOS, A.S.pt_BR
dc.contributor.authorSOUZA, R.F.B. dept_BR
dc.contributor.authorOLIVEIRA NETO, A.pt_BR
dc.coverageInternacionalpt_BR
dc.date.accessioned2021-03-23T13:14:26Z
dc.date.available2021-03-23T13:14:26Z
dc.date.issued2021pt_BR
dc.description.abstractPdxCuy/C catalysts combinations were employed to CH4 partial oxidation in mild condition using a solid electrolyte reactor—alkaline fuel cell type. The differential mass spectroscopy on line method was used to monitor the oxidation products obtained as methanol, dimethyl ether, methyl formate and potassium formate. It was observed that as the electrical potential of the reactor increases, the generation of products decreases. The best results for conversion of methane into methanol and energy co-generation was obtained from Pd90Cu10/ C and Pd50Cu50/ C due to better H2O activation effects and adsorption site for CH4 oxidation.pt_BR
dc.description.sponsorshipConselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq)pt_BR
dc.description.sponsorshipFundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)pt_BR
dc.description.sponsorshipIDCNPq: 300816/2016-2pt_BR
dc.description.sponsorshipIDFAPESP: 14/09087-4; 14/50279-4; 17/11937-4; 17/11937-4pt_BR
dc.format.extent743-757pt_BR
dc.identifier.citationGODOI, C.M.; SANTOS, M.C.L.; SILVA, A.J.; TAGOMORI, T.L.; RAMOS, A.S.; SOUZA, R.F.B. de; OLIVEIRA NETO, A. Methane conversion to higher value‑added product and energy co‑generation using anodes OF PdCu/C in a solid electrolyte reactor: alkaline fuel cell type monitored by differential mass spectroscopy. <b>Research on Chemical Intermediates</b>, v. 47, n. 2, p. 743-757, 2021. DOI: <a href="https://dx.doi.org/10.1007/s11164-020-04296-4">10.1007/s11164-020-04296-4</a>. Disponível em: http://repositorio.ipen.br/handle/123456789/31938.
dc.identifier.doi10.1007/s11164-020-04296-4pt_BR
dc.identifier.fasciculo2pt_BR
dc.identifier.issn0922-6168pt_BR
dc.identifier.orcid0000-0001-8745-3421pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-9287-6071
dc.identifier.percentilfi46.09pt_BR
dc.identifier.percentilfiCiteScore70.00
dc.identifier.urihttp://repositorio.ipen.br/handle/123456789/31938
dc.identifier.vol47pt_BR
dc.relation.ispartofResearch on Chemical Intermediatespt_BR
dc.rightsopenAccesspt_BR
dc.subjectmethane
dc.subjectelectrocatalysts
dc.subjectsolid electrolytes
dc.subjectoxidation
dc.subjectmethanol
dc.subjectfourier transformation
dc.subjectinfrared spectra
dc.subjectmass spectroscopy
dc.titleMethane conversion to higher value‑added product and energy co‑generation using anodes OF PdCu/C in a solid electrolyte reactorpt_BR
dc.typeArtigo de periódicopt_BR
dspace.entity.typePublication
ipen.autorARACELI JARDIM SILVA
ipen.autorRODRIGO FERNANDO BRAMBILLA DE SOUZA
ipen.autorALMIR OLIVEIRA NETO
ipen.autorANDREZZA DA SILVA RAMOS
ipen.autorMONIQUE CAROLINA LIMA DOS SANTOS
ipen.autorCAMILA MARINHO GODOI SANTOS
ipen.codigoautor15469
ipen.codigoautor11260
ipen.codigoautor3541
ipen.codigoautor15158
ipen.codigoautor14122
ipen.codigoautor14128
ipen.contributor.ipenauthorARACELI JARDIM SILVA
ipen.contributor.ipenauthorRODRIGO FERNANDO BRAMBILLA DE SOUZA
ipen.contributor.ipenauthorALMIR OLIVEIRA NETO
ipen.contributor.ipenauthorANDREZZA DA SILVA RAMOS
ipen.contributor.ipenauthorMONIQUE CAROLINA LIMA DOS SANTOS
ipen.contributor.ipenauthorCAMILA MARINHO GODOI SANTOS
ipen.date.recebimento21-03
ipen.identifier.fi3.134pt_BR
ipen.identifier.fiCiteScore5.0
ipen.identifier.ipendoc27709pt_BR
ipen.identifier.iwosWoSpt_BR
ipen.identifier.ods7
ipen.range.fi3.000 - 4.499
ipen.range.percentilfi25.00 - 49.99
ipen.subtituloalkaline fuel cell type monitored by differential mass spectroscopypt_BR
ipen.type.genreArtigo
relation.isAuthorOfPublication41b71c5e-d9b3-4e0e-888f-4c5a95274331
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sigepi.autor.atividadeOLIVEIRA NETO, A.:3541:610:Npt_BR
sigepi.autor.atividadeSOUZA, R.F.B. de:11260:610:Npt_BR
sigepi.autor.atividadeRAMOS, A.S.:15158:610:Npt_BR
sigepi.autor.atividadeSILVA, A.J.:15469:610:Npt_BR
sigepi.autor.atividadeSANTOS, M.C.L.:14122:610:Npt_BR
sigepi.autor.atividadeGODOI, C.M.:14128:610:Spt_BR
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